Light Quanta · Paper 1, §7 Energy Conservation

Stokes's Rule and the Single-Quantum Energy Budget

Why the frequency of emitted fluorescent light cannot exceed that of the exciting light under elementary quantum transformation, and how Einstein deduced the exact conditions for exceptions.

Light Quanta · §7 Fluorescence & Stokes's Rule

Fluorescence Energy Budget & Stokes's Rule

How single-quantum energy conservation hν₁ = hν₂ + E_other explains Stokes's rule (ν₂ ≤ ν₁) and correctly predicts multi-quantum and thermal deviation conditions.

Predict Mode · Energy Conservation

Can fluorescent emission occur at higher frequency than the exciting light (ν₂ > ν₁) under single-quantum absorption?

Predict Mode · Weak-Illumination Linearity

How does the emission rate behave as the incident light becomes extremely weak?

Elementary Quantum Energy LedgerAllowed by Budget
Stokes's Rule (§7)
0 eV (Ground State)3.515 eVAbsorbed (hν₁)850 THz · 353 nmν₂,max = 850.0 THz3.515 eVEmitted (hν₂)850 THz · 353 nm+0.000 eVHeat (E_other)Dissipated in medium
Verdict: Allowed under Stokes's rule: emitted quantum energy does not exceed absorbed quantum energy (nu2 <= nu1).

Spectral Bands & False-Color Legend

Wavelength λ = c / ν
Ultraviolet (UV)
> 789 THz (< 380 nm)
Visible Spectrum
400–789 THz (380–750 nm)
Infrared (IR)
< 400 THz (> 750 nm)
Weak-Illumination Photon Rates (Zero Threshold)Yield Y = 0.50
Absorbed Rate Ṅ₁:1.7755e+12 s⁻¹
Emitted Rate Ṅ₂:8.8776e+11 s⁻¹
Emitted Power:0.5000 μW
Heat Dissipated:0.5000 μW

Interactive Energy & Parameter Controls

THz(3.515 eV)
THz(3.515 eV)
Accounting Regime:
Available Channels:

Calculated Energy Ledger & Transition Quantities

Physical QuantitySymbolCalculated ValuePhysical Meaning
Budget VerdictVerdictAllowedAllowed under Stokes's rule: emitted quantum energy does not exceed absorbed quantum energy (nu2 <= nu1).
Maximum Allowed Frequencyν₂,max850.00 THzUpper frequency bound for emitted light
Absorbed Quantum Energyhν₁3.5153 eVEnergy of one exciting light quantum
Emitted Quantum Energyhν₂3.5153 eVEnergy of candidate emitted light quantum
Non-Optical Dissipation (Heat)E_other0.0000 eVEnergy transferred to thermal modes of medium
Energy DeficitΔE0.0000 eVZero (Conserved)

Paper Assumptions (§7 as printed)

  • The exciting light consists of energy quanta of magnitude h*nu1 as derived for the Wien regime.
  • The absorption and emission of light are elementary processes occurring via single quanta (unless in deviation case 1).
  • Each absorbed quantum is transformed into a light quantum of frequency nu2 and/or non-optical energy channels (heat).
  • Energy is strictly conserved in every elementary transformation: h*nu1 = h*nu2 + E_other with E_other >= 0.

What this model leaves out (not modeled)

  • Detailed atomic or molecular energy level structures and transition dipoles.
  • Non-radiative decay kinetics and intermediate triplet states (phosphorescence timescales).
  • Spatial propagation, self-absorption, and re-emission geometry inside the bulk medium.
  • Coherent optical effects and laser amplification.

The Single-Quantum Energy Budget in Einstein 1905 §7

In 1852, George Gabriel Stokes formulated the empirical rule that fluorescent light always has a lower frequency (longer wavelength) than the light that excited it. In §7 of his 1905 paper, Einstein showed that this rule is an immediate consequence of the light-quantum hypothesis:

“If monochromatic light of frequency ν₁ is transformed into light of frequency ν₂ by photoluminescence, and if the process occurs such that one absorbed quantum is converted into one emitted quantum plus non-optical energy... then the energy of the emitted quantum cannot be greater than that of the exciting one.”
hν₁ = hν₂ + E_other  (E_other ≥ 0)  &Longrightarrow;  ν₂ ≤ ν₁

The Two Historical Deviation Cases

Rather than stating Stokes's rule as an unbreakable law, Einstein explicitly deduced the physical conditions under which anti-Stokes emission (ν₂ > ν₁) can occur:

  • Deviation Case 1 (Multi-quantum absorption): If the elementary process involves the simultaneous absorption of k light quanta, the available energy is k hν₁, permitting emission up to ν₂ ≤ k ν₁.
  • Deviation Case 2 (Non-Wien exciting radiation): If the incident light is not in the Wien regime (where the light-quantum volume law was derived), single-quantum behavior is not guaranteed.
Read the original German source text and translation for §7 →